Laura deferred her studies in psychology to continue modelling when she got back home to Australia. Her success continued when she became the first Australian face of international shoe label Steve Madden as well as the official ambassador for both the Spring and Autumn racing carnivals for the Sydney Turf Club. Opening Sydney Fashion Festival for Charlie Brown in 2008 led to Dundovic being signed as this leading Australian designers face. Laura Dundovic continues to work with Charlie Brown and has also been come an ambassador for Myer.
She will host a TV dating show by FoxTel, according to a report in the Daily Telegraph, in which three couples live under one roof but only have contact in a "specially created dark room" -- the show is tentatively titled "Dating in the Dark".
In February 2011, Laura was appointed as the official Ambassador for Hollywood Fashion Tape.